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Paper · arXiv

Human-agent discovery of reconfigurable in-plane ferroelectric superdomain control

Automated experimentation is most effective when the observables, available actions, and objective are defined before the experiment starts, as is the case for Bayesian optimization. However, in many exploratory experiments, the variables that describe the sample must be extracted from the data, new operations emerge during the experiments, and the instrument budget is too small to learn the problem by trials. Here we introduce the Scanning Probe Agentic Research Cycle (SPARC) framework, in which a coding agent and a human operator share one microscope, one notebook, and two persistent memory files. FINDINGS.md stores graded conclusions about the experiment, whereas PITFALLS.md records le...

AuthorsYu Liu, Boris Slautin, Ching-Che Lin et al.
Primary categorycond-mat.mtrl-sci
Published7 September 2026
Last updated at source7 September 2026
cond-mat.mtrl-scics.AI
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